Design and Analysis for Melt Casting Metallic Fuel pins Incorporating Volatile
Actinides The development of higher actinide transmutation fuels systems presents
a challenge for many scientists and engineers. Fuel must behave in a benign
manner during reactor off-normal events, maintain integrity to high burnup,
lend itself to low-loss recycling processes, and be easily fabricated in a
remote environment. These criteria are important for a fuel to perform and
function efficiently and effectively within a transmutation system. Currently,
engineers and scientists do not have enough data to design and optimize the
selection of a fuel system. The fundamental design and analysis for fuel system
and fabrication research are needed to lay the groundwork for future fuel
development. The Accelerator-driven Transmutation of Waste (ATW) program has
listed several critical issues in fuel requirements: cladding integrity, fission
product retention, and dimensional, chemical, and metallurgical stability
during irradiation under both normal and off-normal conditions. Volatile actinide
elements, such as americium, can be easily incorporated into metallic alloy
fuel pins under traditional casting process using inductively heated crucible.
The traditional casting process performs well for fabrication of metal fuel
pins composed of alloys, including uranium and plutonium. However, it is not
suitable when high volatile actinides are present in the melted mixture. Low-pressure
actinides, particularly americium, are susceptible to rapid vaporization and
transport throughout the casting furnace, resulting in a fraction of the charge
being incorporated into the fuel pins as desired. A robust casting process
for the metallic fuel pins containing volatile actinides will be evaluated
and developed. The design and analysis for melt casting metallic fuel pins
incorporating volatile actinides will be focused on selecting, evaluating,
and modeling potential alternatives to traditional injection casting processes
already in use at the Argonne National Laboratory. Processing conditions,
basic models utilization, and detailed of heat and mass transfer models will
also be developed and analyzed.